Synthesis of Co2[Fe(CN)6]/g-C3N4 composite as an improved photocatalyst for degradation of methylene blue

Authors: Vo Nhu Quynh; Do Hoang Chinh; Nguyen Thi Quynh Giao; Tran Thi Thanh Tuyen; Tran Thi Phuong Diem; Pham Ho Khanh Doan; Truong Cong Duc; Le Thi Thanh Lieu; Nguyen Thi Viet Nga; Nguyen Van Kim
Journal: Quy Nhon University Journal of Science
Published: 2026/02/28
Volume/Issue: Vol. 20, Issue 1
Pages: 59-69
DOI: https://doi.org/10.52111/qnjs.2026.20106

Abstract

In this study, the Co 2 [Fe(CN) 6 ]/ g -C 3 N 4 composite was synthesized by first preparing g-C 3 N 4 and Co 2 [Fe(CN) 6 ] separately, followed by their coupling through the dispersion of Co 2 [Fe(CN) 6 ] onto g-C 3 N 4 at 90 o C for 1 hour. The resulting materials were characterized by X-ray diffraction (XRD), Fourier-transform infrared spectroscopy (FT-IR), energy-dispersive X-ray spectroscopy (EDS), scanning electron microscopy (SEM), UV-Vis diffuse reflectance spectroscopy (UV-Vis DRS), and photoluminescence (PL) spectroscopy. The photocatalytic performance of the composite was evaluated via the degradation of methylene blue (MB) in aqueous solution under sunlight irradiation. The Co 2 [Fe(CN) 6 ]/ g -C 3 N 4 composite exhibited superior photocatalytic activity compared to the individual components, g-C 3 N 4 and Co 2 [Fe(CN) 6 ] .

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